Tailored Raman-resonant four-wave-mixing process

Nonlinear optical processes are strongly dominated by phase relationships among electromagnetic fields that are relevant to its optical process. In this paper, we theoretically and experimentally show, as a typical example, that in a Raman-resonant four-wave-mixing process, the first anti-Stokes and Stokes generations can be tailored to a variety of forms by manipulating the phase relationships among the relevant electromagnetic fields.