Theoretical Modeling of the Non-equilibrium Amorphous State in 1T-TaS₂
classification
❄️ cond-mat.str-el
keywords
stateamorphousbeenmetastablephaset-tasbrazovskiicase
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1T-TaS$_2$ is known for it's remarkably complex phase diagram and it's unique long-lived metastable hidden (H) state. Recently, a novel metastable state has been discovered using higher fluences for photoexcitation than in the case of the H state. The state has been dubbed as amorphous (A) due to it's similarity to glass. Expanding on the work of Brazovskii and Karpov, we show that the A state can be successfully modelled with classical interacting polarons on a two-dimensional hexagonal lattice. We have found that the polaron configuration of the A state corresponds to a frustrated screened Coulomb system, where there is no order-disorder phase transition.
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