Inhomogeneous CuO₆ Tilt Distribution and Charge/Spin Correlations in La_(2-x-y)Nd_(y)Sr_(x)CuO₄ around commensurate hole concentration
classification
❄️ cond-mat.str-el
keywords
aroundchargeconcentrationdisorderdopingramanscatteringspin
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Phononic and magnetic Raman scattering are studied in La$_{2-x-y}$Nd$_{y}$Sr$_{x}$CuO$_{4}$ with three doping concentrations: x ~ 1/8, y = 0; x ~ 1/8, y = 0.4; and x = 0.01, y = 0. We observe strong disorder in the tilt pattern of the CuO_{6} octahedra in both the orthorhombic and tetragonal phases which persist down to 10 K and are coupled to bond disorder in the cation layers around 1/8 doping independent of Nd concentration. The weak magnitude of existing charge/spin modulations in the Nd doped structure does not allow us to detect the specific Raman signatures on lattice dynamics or two-magnon scattering around 2200 cm-1.
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