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arxiv: cond-mat/0401536 · v1 · submitted 2004-01-27 · ❄️ cond-mat.dis-nn

Nearly-logarithmic decay of correlations in glass-forming liquids

classification ❄️ cond-mat.dis-nn
keywords correlationsdecayfluctuationslettliquidsnearly-logarithmicphysagreement
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Nearly-logarithmic decay of correlations, which was observed for several supercooled liquids in optical-Kerr-effect experiments [G. Hinze et al. Phys. Rev. Lett. 84, 2437(2000), H. Cang et al. Phys. Rev. Lett. 90, 197401 (2003)], is explained within the mode-coupling theory for ideal glass transitions as manifestation of the $\beta$-peak phenomenon. A schematic model, which describes the dynamics by only two correlators, one referring to density fluctuations and the other to the reorientational fluctuations of the molecules, yields for strong rotation-translation coupling response functions in agreement with those measured for benzophenone and Salol for the time interval extending from 2 picoseconds to about 20 and 200 nanoseconds, respectively.

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