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arxiv: cond-mat/0402586 · v2 · submitted 2004-02-24 · ❄️ cond-mat.str-el

Intrinsic susceptibility and bond defects in the novel 2D frustrated antiferromagnet Ba₂Sn₂ZnCr_(7p)Ga_(10-7p)O₂₂

classification ❄️ cond-mat.str-el
keywords bonddefectsfrustratedmagneticsusceptibilityantiferromagnetdilutionintrinsic
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We present microscopic and macroscopic magnetic properties of the highly frustrated antiferromagnet Ba$_{2}$Sn$_{2}$ZnCr$_{7p}$Ga$_{10-7p}$O$_{22}$, respectively probed with NMR and SQUID experiments. The $T$-variation of the intrinsic susceptibility of the Cr$^{3+}$ frustrated kagom\'{e} bilayer, $\chi_{kag}$, displays a maximum around 45 K. The dilution of the magnetic lattice has been studied in detail for $0.29 \leq p \leq0.97$. Novel dilution independent defects, likely related with magnetic bond disorder, are evidenced and discussed. We compare our results to SrCr$_{9p}$Ga$_{12-9p}$O$_{19}$. Both bond defects and spin vacancies do not affect the average susceptibility of the kagom\'{e} bilayers.

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