Electromagnetic response of broken-symmetry nano-scale clusters
classification
❄️ cond-mat.str-el
keywords
clusterselectromagneticnano-scaleresponsetheorybelowbreakdownbroken-symmetry
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A microscopic, non-local response theory is developed to model the interaction of electromagnetic radiation with inhomogeneous nano-scale clusters. The breakdown of classical continuum-field Mie theory is demonstrated at a critical coarse-graining threshold, below which macroscopic plasmon resonances are replaced by molecular excitations with suppressed spectral intensity.
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