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Generic spin model for the honeycomb iridates beyond the Kitaev limit

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arxiv 1310.7940 v3 pith:32GMQ3JG submitted 2013-10-29 cond-mat.str-el

classification cond-mat.str-el
keywords kitaevexchangemodeldirectgenericheisenberghoneycombiridates
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Recently, realizations of Kitaev physics have been sought in the A2IrO3 family of honeycomb iridates, originating from oxygen-mediated exchange through edge-shared octahedra. However, for the j = 1/2 Mott insulator in these materials exchange from direct d-orbital overlap is relevant, and it was proposed that a Heisenberg term should be added to the Kitaev model. Here we provide the generic nearest-neighbour spin Hamiltonian when both oxygen-mediated and direct overlap are present, containing a bond dependent off-diagonal exchange in addition to Heisenberg and Kitaev terms. We analyze this complete model using a combination of classical techniques and exact diagonalization. Near the Kitaev limit, we find new magnetic phases, 120 degree and incommensurate spiral order, as well as extended regions of zigzag and stripy order. Possible applications to Na2IrO3 and Li2IrO3 are discussed.

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  1. Weak ergodicity breaking with isolated integrable sectors

    cond-mat.stat-mech 2024-12 accept novelty 7.0 of 10

    Isolated integrable subspaces can be embedded non-trivially into chaotic spin chains; all examples are perturbations of Hilbert-space-fragmented models.

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