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Pressure-induced melting of magnetic order and emergence of new quantum state in alpha-RuCl3

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arxiv 1705.06139 v2 pith:K3MSOXWB submitted 2017-05-17 cond-mat.str-el

classification cond-mat.str-el
keywords quantumstatehigh-pressureorderphasepressurealpha-rucl3emergence
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Here we report the observation of pressure-induced melting of antiferromagnetic (AFM) order and emergence of a new quantum state in the honeycomb-lattice halide alpha-RuCl3, a candidate compound in the proximity of quantum spin liquid state. Our high-pressure heat capacity measurements demonstrate that the AFM order smoothly melts away at a critical pressure (Pc) of 0.7 GPa. Intriguingly, the AFM transition temperature displays an increase upon applying pressure below the Pc, in stark contrast to usual phase diagrams, for example in pressurized parent compounds of unconventional superconductors. Furthermore, in the high-pressure phase an unusual steady of magnetoresistance is observed. These observations suggest that the high-pressure phase is in an exotic gapped quantum state which is robust against pressure up to ~140 GPa.

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  1. Electronic properties of {\alpha}-RuCl3 in proximity to graphene

    cond-mat.str-el 2019-08 conditional novelty 6.0 of 10

    In α-RuCl3/graphene heterostructures, DFT calculations predict charge transfer and tensile strain that metallize α-RuCl3 and enhance its Kitaev coupling by more than 50% compared with bulk.

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