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Reconstruction of attosecond pulses in the presence of interfering dressing fields using the 100 kHz ELI-ALPS HR-1 laser system

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arxiv 1906.07059 v1 pith:2BQWBZAI submitted 2019-06-17 physics.atom-ph

classification physics.atom-ph
keywords attosecondlaserrabbitbeatingeli-alpsexperimentsmeasurementsfirst
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Attosecond Pulse Trains (APT) generated by high-harmonic generation (HHG) of high-intensity near-infrared (IR) laser pulses have proven valuable for studying the electronic dynamics of atomic and molecular species. However, the high intensities required for high-photon-energy, high-flux HHG usually limit the class of adequate laser systems to repetition rates below 10~kHz. Here, APT's generated from the 100 kHz, 160 W, 40 fs laser system (HR1) of the Extreme Light Infrastructure Attosecond Light Pulse Source (ELI-ALPS) are reconstructed using the Reconstruction of Attosecond Beating By Interference of two-photon Transitions (RABBIT) technique. These experiments constitute the first attosecond time-resolved photoelectron spectroscopy measurements performed at 100 kHz repetition rate and the first attosecond experiments performed at ELI-ALPS. These RABBIT measurements were taken with an additional IR field temporally locked to the extreme-ultraviolet APT, resulting in an atypical omega beating. We show that the phase of the 2-omega beating recorded under these conditions is strictly identical to that observed in standard RABBIT measurements within second-order perturbation theory. This work highlights an experimental simplification for future experiments based on attosecond interferometry (or RABBIT), which is particularly useful when lasers with high average powers are used.

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  1. Generation and characterization of few-pulse attosecond pulse trains at 100kHz repetition rate

    physics.optics 2019-08 conditional novelty 5.0 of 10

    A 100 kHz NOPCPA driver generates attosecond pulse trains in the extreme ultraviolet, characterized via FROG-CRAB with a retrieved central pulse duration of 240 ± 20 as.

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