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Optical and acoustic plasmons in the layered material Sr$_2$RuO$_4$

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arxiv 2401.05880 v3 pith:5YI4JUM5 submitted 2024-01-11 cond-mat.str-el

classification cond-mat.str-el
keywords energyopticalplasmonacousticexcitationsmetalplasmonsrange
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abstract

We use momentum-dependent electron energy-loss spectroscopy in transmission to study collective charge excitations in the layer metal Sr$_2$RuO$_4$. This metal has a transition from a perfect Fermi liquid below $T\approx30\,$K into a "strange" metal phase above $T\approx800\,$K. We cover a complete range between in-phase and out-of-phase oscillations. Outside the classical range of electron-hole excitations, leading to a Landau damping, we observe well-defined plasmons. The optical (acoustic) plasmon due to an in-phase (out-of-phase) charge oscillation of neighbouring layers exhibits a quadratic (linear) positive dispersion. Using a model for the Coulomb interaction of the charges in a layered system, it is possible to describe the range of optical plasmon excitations at high energies in a mean-field random phase approximation without taking correlation effects into account. In contrast, resonant inelastic X-ray scattering data show at low energies an enhancement of the acoustic plasmon velocity due to correlation effects. This difference can be explained by an energy dependent effective mass which changes from $\approx$ 3.5 at low energy to 1 at high energy near the optical plasmon energy. There are no signs of over-damped plasmons predicted by holographic theories.

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  1. Unconventional Materials for Light Dark Matter Detection

    hep-ph 2025-07 conditional novelty 6.0 of 10

    TiSe2, Sr2RuO4, and hole-doped diamond are projected to improve sub-MeV dark matter detection reaches by one to three orders of magnitude over existing proposals, with directional sensitivity from their anisotropic responses.

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