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Incommensurate broken helix induced by nonstoichiometry in the axion insulator candidate EuIn$_{2}$As$_{2}$
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abstract
Zintl phase EuIn$_{2}$As$_{2}$ has garnered growing attention as an axion insulator candidate, triggered by the identification of a commensurate double-${\mathbf Q}$ broken-helix state in previous studies, however, its periodicity and symmetry remain subjects of debate. Here, we perform resonant x-ray scattering experiments on EuIn$_{2}$As$_{2}$, revealing an incommensurate nature of the broken-helix state, where both the wave number and the amplitude of the helical modulation exhibit systematic sample dependence. Furthermore, the application of an in-plane magnetic field brings about a fanlike state that appears to preserve the double-${\mathbf Q}$ nature, which might be attributed to multiple-spin interactions in momentum space. We propose that the itinerant character of EuIn$_{2}$As$_{2}$, most likely induced by Eu deficiency, gives rise to the helical modulation and impedes the realization of a theoretically-predicted axion state with the collinear antiferromagnetic order.
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Cited by 2 Pith papers
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Goldstone mode of the broken helix in U(1) magnet EuIn2As2
The Goldstone mode frequency in the broken-helix magnet EuIn2As2 scales linearly with in-plane magnetic field, matching a symmetry-based prediction for C2z-symmetric magnets.
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Non-relativistic linear Edelstein effect in helical EuIn2As2
In the helical and broken-helical phases of EuIn2As2, magnetic exchange creates non-relativistic spin textures that yield a phase-distinguishing Edelstein response, about five times larger in the helical phase.
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