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Incommensurate broken helix induced by nonstoichiometry in the axion insulator candidate EuIn$_{2}$As$_{2}$

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arxiv 2403.03022 v2 pith:MMIXFR33 submitted 2024-03-05 cond-mat.str-el

classification cond-mat.str-el
keywords euinstateaxionbroken-helixcandidatedouble-helicalincommensurate
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abstract

Zintl phase EuIn$_{2}$As$_{2}$ has garnered growing attention as an axion insulator candidate, triggered by the identification of a commensurate double-${\mathbf Q}$ broken-helix state in previous studies, however, its periodicity and symmetry remain subjects of debate. Here, we perform resonant x-ray scattering experiments on EuIn$_{2}$As$_{2}$, revealing an incommensurate nature of the broken-helix state, where both the wave number and the amplitude of the helical modulation exhibit systematic sample dependence. Furthermore, the application of an in-plane magnetic field brings about a fanlike state that appears to preserve the double-${\mathbf Q}$ nature, which might be attributed to multiple-spin interactions in momentum space. We propose that the itinerant character of EuIn$_{2}$As$_{2}$, most likely induced by Eu deficiency, gives rise to the helical modulation and impedes the realization of a theoretically-predicted axion state with the collinear antiferromagnetic order.

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Cited by 2 Pith papers

Reviewed papers in the Pith corpus that reference this work. Sorted by Pith novelty score. Full citation record

  1. Goldstone mode of the broken helix in U(1) magnet EuIn2As2

    cond-mat.mtrl-sci 2025-01 conditional novelty 7.0 of 10

    The Goldstone mode frequency in the broken-helix magnet EuIn2As2 scales linearly with in-plane magnetic field, matching a symmetry-based prediction for C2z-symmetric magnets.

  2. Non-relativistic linear Edelstein effect in helical EuIn2As2

    cond-mat.str-el 2024-12 conditional novelty 6.0 of 10

    In the helical and broken-helical phases of EuIn2As2, magnetic exchange creates non-relativistic spin textures that yield a phase-distinguishing Edelstein response, about five times larger in the helical phase.

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