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Field-tunable quantum disordered ground state in the triangular lattice antiferromagnet NaYbO$_2$

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arxiv 1901.09408 v2 pith:7QZ4HNTX submitted 2019-01-27 cond-mat.str-el cond-mat.other

classification cond-mat.str-elcond-mat.other
keywords quantumstategroundlatticeliquidspintriangulardisordered
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abstract

Antiferromagnetically coupled S=1/2 spins on an isotropic triangular lattice is the paradigm of frustrated quantum magnetism, but structurally ideal realizations are rare. Here we investigate NaYbO$_2$, which hosts an ideal triangular lattice of $J_{eff}=1/2$ moments with no inherent site disorder. No signatures of conventional magnetic order appear down to 50 mK, strongly suggesting a quantum spin liquid ground state. We observe a two-peak specific heat and a nearly quadratic temperature dependence in accord with expectations for a two-dimensional Dirac spin liquid. Application of a magnetic field strongly perturbs the quantum disordered ground state and induces a clear transition into a collinear ordered state consistent with a long-predicted up-up-down structure for a triangular lattice XXZ Hamiltonian driven by quantum fluctuations. The observation of spin liquid signatures in zero field and quantum-induced ordering in intermediate fields in the same compound demonstrate an intrinsically quantum disordered ground state. We conclude that NaYbO$_2$ is a model, versatile platform for exploring spin liquid physics with full tunability of field and temperature.

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  1. Single-site magnetic anisotropy governed by inter-layer cation charge imbalance in triangular-lattice AYbX$_2$

    cond-mat.str-el 2019-09 conditional novelty 6.0 of 10

    The strongly anisotropic g factors of Yb3+ in NaYbS2 and NaYbO2 are controlled mainly by the charge contrast between in-plane Yb3+ neighbors and inter-layer Na+ ions, with a more homogeneous cation environment yieldin...

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