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arxiv: 1004.1468 · v1 · pith:AOWBTL4Mnew · submitted 2010-04-09 · ⚛️ physics.atom-ph

Ionization of oriented targets by intense circularly polarized laser pulses: Imprints of orbital angular nodes in the 2D momentum distribution

classification ⚛️ physics.atom-ph
keywords circularlyorbitalpolarizedpulseresultsstateangularinitial
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We solve the three-dimensional time-dependent Schr\"{o}dinger equation for a few-cycle circularly polarized femtosecond laser pulse interacting with an oriented target exemplified by an Argon atom, initially in a $3\text{p}_{x}$ or $3\text{p}_{y}$ state. The photoelectron momentum distributions show distinct signatures of the orbital structure of the initial state as well as the carrier-envelope phase of the applied pulse. Our \textit{ab initio} results are compared with results obtained using the length-gauge strong-field approximation, which allows for a clear interpretation of the results in terms of classical physics. Furthermore, we show that ionization by a circularly polarized pulse completely maps out the angular nodal structure of the initial state, thus providing a potential tool for studying orbital symmetry in individual systems or during chemical reactions.

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