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Antiferromagnetic ordering and dipolar interactions of YbAlO$_3$

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arxiv 1904.11513 v2 pith:BNJBREOW submitted 2019-04-25 cond-mat.str-el

classification cond-mat.str-el
keywords momentsalongmagneticybaloantiferromagneticaxisinteractionneutron
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abstract

In this paper we report low-temperature magnetic properties of the rare-earth perovskite material YbAlO$_3$. Results of elastic and inelastic neutron scattering experiment, magnetization measurements along with the crystalline electrical field (CEF) calculations suggest that the ground state of Yb moments is a strongly anisotropic Kramers doublet, and the moments are confined in the $ab$-plane, pointing at an angle of $\varphi = \pm 23.5^{\circ}$ to the $a$-axis. With temperature decreasing below $T_{\rm N}=0.88$ K, Yb moments order into the coplanar, but non-collinear antiferromagnetic (AFM) structure $AxGy$, where the moments are pointed along their easy-axes. In addition, we highlight the importance of the dipole-dipole interaction, which selects the type of magnetic ordering and may be crucial for understanding magnetic properties of other rare-earth orthorhombic perovskites. Further analysis of the broad diffuse neutron scattering shows that one-dimensional interaction along the $c$-axis is dominant, and suggests YbAlO$_3$ as a new member of one dimensional quantum magnets.

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  1. Phase diagram and quantum criticality of Heisenberg spin chains with Ising-like interchain couplings -- Implication to YbAlO$_3$

    cond-mat.str-el 2019-08 conditional novelty 6.0 of 10

    Quantum Monte Carlo shows that Ising-like interchain couplings stabilize an incommensurate longitudinal spin density wave in Heisenberg chains, with a (3+2)D XY quantum critical point at saturation.

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