Polarization conversion of non-specular diffraction orders from metallic nanohole arrays studied by Fourier space polarimetry

We use Fourier space polarimetry to study the incident angle- and polarization-dependent rotation angle and ellipticity of different diffraction orders emerging from a two-dimensional periodic Au array. The array has square lattice and circular nanoholes and thus is achiral. We find no polarization conversion occurs if the diffraction orders lie in the incident plane. However, for the orders that are diffracted away from the incident plane, their rotation angle and ellipticity vary considerably with incident angle and polarization. In particular, dramatic changes in rotation angle and ellipticity are observed when Bloch-like surface plasmon polaritons (SPPs) are excited. The experimental results are consistent with the finite-difference time-domain simulations. The transverse spin carried by the SPPs and a discrete dipole model are used complementarily to elucidate such angular and polarization dependences.