Mutual Experimental and Theoretical Validation of Bulk Photoemission Spectra of Sr1-xCaxVO3

A. Sekiyama; A. V. Kozhevnikov; D. E. Kondakov; D. Vollhardt; G. Keller; H. Eisaki; H. Fujiwara; H. Harima; I. A. Nekrasov; K. Held

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Mutual Experimental and Theoretical Validation of Bulk Photoemission Spectra of Sr1-xCaxVO3

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arxiv cond-mat/0312429 v3 pith:HQS4ERV3 submitted 2003-12-17 cond-mat.str-el

A. Sekiyama , H. Fujiwara , S. Imada , S. Suga , H. Eisaki , S. I. Uchida , K. Takegahara , H. Harima

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Y. Saitoh I. A. Nekrasov G. Keller D. E. Kondakov A. V. Kozhevnikov Th. Pruschke K. Held D. Vollhardt V. I. Anishimov

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keywords spectraphotoemissionbulkhigh-energysr1-xcaxvo3theoryagreementapproximation

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We report high-resolution high-energy photoemission spectra together with parameter-free LDA+DMFT (local density approximation + dynamical mean-field theory) results for Sr1-xCaxVO3, a prototype 3d1 system. In contrast to earlier investigations the bulk spectra are found to be insensitive to x. The good agreement between experiment and theory confirms the bulk-sensitivity of the high-energy photoemission spectra.

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