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arxiv: 2305.03528 · v1 · pith:IE62QUJAnew · submitted 2023-05-05 · ❄️ cond-mat.str-el

Ultrafast all-optical manipulation of the charge-density-wave in VTe₂

classification ❄️ cond-mat.str-el
keywords phasecollectivegroundmodesstateultrafastall-opticalamplitude
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The charge-density wave (CDW) phase in the layered transition-metal dichalcogenide VTe$_{2}$ is strongly coupled to the band inversion involving vanadium and tellurium orbitals. In particular, this coupling leads to a selective disappearance of the Dirac-type states that characterize the normal phase, when the CDW phase sets in. Here, by means of broadband time-resolved optical spectroscopy (TR-OS), we investigate the ultrafast reflectivity changes caused by collective and single particle excitations in the CDW ground state of VTe$_{2}$. Remarkably, our measurements show the presence of two collective (amplitude) modes of the CDW ground state. By applying a double-pulse excitation scheme, we show the possibility to manipulate these modes, demonstrating a more efficient way to control and perturb the CDW phase in VTe$_{2}$.

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