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arxiv: 1904.08044 · v3 · pith:LT2NZGX2new · submitted 2019-04-17 · ⚛️ physics.atom-ph

Correlation enhancement of high-order harmonics generation in Xe

classification ⚛️ physics.atom-ph
keywords correlationenhancementgenerationharmonicshigh-orderinter-shellphysreported
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We consider the process of high-order harmonics generation (HHG) in the xenon atom enhanced by the inter-shell correlation between the valence 5p and inner 4d shells. We derive the HHG spectrum from a numerical solution of the one-electron time-dependent Schr\"odinger equation multiplied by the enhancement factor taken as the photoionization cross-sections ratio calculated with and without the inter-shell correlation. Such a simplified approach is adequate to describe the experimental HHG spectrum reported by Shiner et al [Nat. Phys. 7, 464 (2011)] generated by a single color IR laser. Similarly, we find good agreement when applied to the two-color driven HHG spectra reported by Facciala et al [Phys. Rev. Lett. 117, 093902 (2016)].

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