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Braided Ising spin-tube physics in a purported kagome magnet

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arxiv 2409.07807 v2 pith:OKPZAMPK submitted 2024-09-12 cond-mat.str-el

classification cond-mat.str-el
keywords isingmagneticmodelkagomephysicssimpleaccountalmost-orthogonal
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abstract

The magnetic insulator Nd$_3$BWO$_9$ has been previously proposed to realize the highly frustrated breathing kagome lattice model. We report a combination of single-crystal neutron scattering studies and numerical simulations that debunk this interpretation. We show that it is the inter-plane couplings that determine the physics. To explain the exotic magnetism, we derive a simple one-dimensional Ising model composed of twisted triangular spin-tubes, i.e., triple braids of Ising spin chains with almost-orthogonal anisotropy frames and competing ferro-antiferromagnetic interactions. This model can account for the ground state, excitations, the numerous field-induced fractional magnetization plateau phases and incommensurate magnetic correlations at elevated temperatures. Nd$_3$BWO$_9$ constitutes a rare example where rich magnetic phenomena can be understood and simulated quantitatively in terms of a simple classical Hamiltonian.

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