Investigation of ac-Stark shifts in excited states of dysprosium relevant to testing fundamental symmetries
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We report on measurements of the differential polarizability between the nearly degenerate, opposite parity states in atomic dysprosium at 19797.96 cm$^{-1}$. The differential scalar and tensor polarizabilities due to additional states were measured for the $|M| = 7,...,10$ sublevels in $^{164}$Dy and $^{162}$Dy and determined to be $\bar{\boldsymbol\alpha}_{\scriptscriptstyle BA}^{(0)} = 180\,(45)_\text{stat}\,(8)_\text{sys}$ $\text{mHz}/(\mathrm{V}/\mathrm{cm})^2$ and $\bar{\boldsymbol\alpha}_{\scriptscriptstyle BA}^{(2)} = -163\,(65)_\text{stat}\,(5)_\text{sys}$ $\text{mHz}/(\mathrm{V}/\mathrm{cm})^2$, respectively. The average blackbody radiation induced Stark shift of the Zeeman spectrum was measured around 300 K and found to be $-34(4)$ mHz/K and $+29(4)$ mHz/K for $^{164}$Dy and $^{162}$Dy, respectively. We conclude that ac-Stark related systematics will not limit a search for variation of the fine-structure constant, using dysprosium, down to the level of $|\dot{\alpha}/\alpha|=2.6\times10^{-17}$ yr$^{-1}$, for two measurements of the transition frequency one year apart.
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