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arxiv: 1506.09185 · v2 · pith:S6S6IL7Dnew · submitted 2015-06-30 · ❄️ cond-mat.str-el

Phase Diagram and Quantum Order by Disorder in the Kitaev K₁-K₂ Honeycomb Magnet

classification ❄️ cond-mat.str-el
keywords kitaevquantumclassicalcouplingdifferenthoneycombmodelphase
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We show that the topological Kitaev spin liquid on the honeycomb lattice is extremely fragile against the second-neighbor Kitaev coupling $K_2$, which has recently been shown to be the dominant perturbation away from the nearest-neighbor model in iridate Na$_2$IrO$_3$, and may also play a role in $\alpha$-RuCl$_3$ and Li$_2$IrO$_3$. This coupling naturally explains the zigzag ordering (without introducing unrealistically large longer-range Heisenberg exchange terms) and the special entanglement between real and spin space observed recently in Na$_2$IrO$_3$. Moreover, the minimal $K_1$-$K_2$ model that we present here holds the unique property that the classical and quantum phase diagrams and their respective order-by-disorder mechanisms are qualitatively different due to the fundamentally different symmetries of the classical and quantum counterparts.

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