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arxiv: 2004.10636 · v3 · pith:SB5NJ4ERnew · submitted 2020-04-22 · ❄️ cond-mat.str-el

Magnetic phase diagram of the linear quantum ferro-antiferromagnet Cs₂Cu₂Mo₃O₁₂

classification ❄️ cond-mat.str-el
keywords phasemagneticdiagramfieldmeasurementsquantumalongbelow
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A single-crystal sample of the frustrated quasi one-dimensional quantum magnet Cs$_{2}$Cu$_{2}$Mo$_{3}$O$_{12}$ is investigated by magnetic and thermodynamic measurements.A combination of specific heat and magnetic torque measurements maps out the entire $H$-$T$ phase diagram for three orientations.Remarkably, a new phase emerges below the saturation field, irrespective of the crystal orientation. It is suggested that the presaturation phase represents spin-nematic order or other multi-magnon condensate. The phase diagrams within the long-range ordered dome are qualitatively different for each geometry. In particular, multiple transitions are identified in the field along the chain direction.

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