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arxiv: 1709.02566 · v1 · pith:TTB5HVHRnew · submitted 2017-09-08 · ❄️ cond-mat.str-el

Evolution of the partially frustrated magnetic order in CePd_(1-x)Ni_xAl

classification ❄️ cond-mat.str-el
keywords magneticapproxcepdconcentrationsevolutionfrustrationorderstructure
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We report on a single-crystal neutron diffraction study of the evolution of the antiferromagnetic order in the heavy-fermion compound CePd$_{1-x}$Ni$_x$Al which exhibits partial geometric frustration due to its distorted Kagom\'e structure. The magnetic structure is found to be unchanged with a propagation vector $Q_\mathrm{AF} \approx (0.5~0~0.35)$ for all Ni concentrations $x$ up to $x_c \approx 0.14$. Upon approaching the quantum critical concentration $x_c$, the ordered moment vanishes linearly with N\'eel temperature $T_{\rm N}$, in good agreement with CePdAl under hydrostatic pressure. For all Ni concentrations, substantial short-range magnetic correlations are observed above $T_{\rm N}$ as a result of frustration.

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