Spectral Peak Recovery in Parametrically Amplified THz-Repetition-Rate Bursts

Multi-photon resonant spectroscopies require tunable narrowband excitation to deliver spectral selectivity and, simultaneously, high temporal intensity to drive a nonlinear-optical process. These contradictory requirements are achievable with bursts of ultrashort pulses, which provides both high intensity and tunable narrowband peaks in the frequency domain arising from spectral interference. However, femtosecond pulse bursts need special attention during their amplification [Optica 7, 1758 (2020)], which requires spectral peak suppression to increase the energy safely extractable from a chirped-pulse amplifier (CPA). Here, we present a method combining safe laser CPA, relying on spectral scrambling, with a parametric frequency converter that automatically restores the desired spectral peak structure and delivers narrow linewidths for bursts of ultrashort pulses at microjoule energies. The shown results pave the way to new high-energy ultrafast laser sources with controllable spectral selectivity.