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Temperature dependent d-d excitations in manganites probed by resonant inelastic x-ray scattering

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arxiv cond-mat/0407326 v1 pith:YUBQ2ITI submitted 2004-07-13 cond-mat.str-el

S. Grenier , J. P. Hill , V. Kiryukhin , W. Ku , Y.-J. Kim , K. J. Thomas , S-W. Cheong , Y. Tokura
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Y. Tomioka D. Casa T. Gog
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classification cond-mat.str-el
keywords excitationstemperaturedependencedependentfoundfunctioninelasticmanganites
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We report the observation of temperature dependent electronic excitations in various manganites utilizing resonant inelastic x-ray scattering (RIXS) at the Mn K-edge. Excitations were observed between 1.5 and 16 eV with temperature dependence found as high as 10 eV. The change in spectral weight between 1.5 and 5 eV was found to be related to the magnetic order and independent of the conductivity. On the basis of LDA+U and Wannier function calculations, this dependence is associated with intersite d-d excitations. Finally, the connection between the RIXS cross-section and the loss function is addressed.

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