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Interplay between quadrupolar and magnetic interactions in 5$d^{1}$ double perovskite Ba$_2$MgReO$_6$ under pressure

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arxiv 2111.09661 v1 pith:Z7CQZ7J7 submitted 2021-11-18 cond-mat.str-el

classification cond-mat.str-el
keywords antiferromagneticmgreoorderpressurecollineardoublemagneticperovskite
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abstract

We measured the electrical resistivity, AC magnetic susceptibility, and specific heat of the cubic double perovskite Ba$_2$MgReO$_6$ under pressure. The application of pressure leads to a gradual increase in the transition temperature to the canted antiferromagnetic order, while the quadrupolar order is suppressed above 5 GPa, at which a collinear antiferromagnetic state appears. The obtained unit cell volume-temperature phase diagram for the compound as well as the related compounds suggests that Ba$_2$MgReO$_6$ exists near the phase boundary between the noncollinear and the collinear antiferromagnetic order with multipole decrees of freedom.

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