Multi-microjoule GaSe-based mid-infrared optical parametric amplifier with an ultra-broad idler spectrum covering 4.2-16 {μ}m

We report a multi-microjoule, ultra-broadband mid-infrared optical parametric amplifier based on a GaSe nonlinear crystal pumped at ~2 {\mu}m. The generated idler pulse has a flat spectrum spanning from 4.5 to 13.3 {\mu}m at -3 dB and 4.2 to 16 {\mu}m in the full spectral range, with a central wavelength of 8.8 {\mu}m. The proposed scheme supports a sub-cycle Fourier-transform-limited pulse width. A (2+1)-dimensional numerical simulation is employed to reproduce the obtained idler spectrum. To our best knowledge, this is the broadest -3 dB spectrum ever obtained by optical parametric amplifiers in this spectral region. The idler pulse energy is ~3.4 {\mu}J with a conversion efficiency of ~2% from the ~2 {\mu}m pump to the idler pulse.