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arxiv: cond-mat/0608442 · v1 · submitted 2006-08-19 · ❄️ cond-mat.str-el

In-Gap Spin Excitations and Finite Triplet Lifetimes in the Dilute Singlet Ground State System SrCu(2-x)Mgx(BO3)2

classification ❄️ cond-mat.str-el
keywords excitationssinglesingletcrystalgroundmagneticspinsrcu
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High resolution neutron scattering measurements on a single crystal of SrCu(2-x)Mgx(BO3)2 with x=0.05 reveal the presence of new spin excitations within the gap of this quasi-two dimensional, singlet ground state system. Application of a magnetic field induces Zeeman-split states associated with S=1/2 unpaired spins which are antiferromagnetically correlated with the bulk singlet. Substantial broadening of both the one and two-triplet excitations in the doped single crystal is observed, as compared with pure SrCu2(BO3)2. Theoretical calculations using a variational algorithm and a single quenched magnetic vacancy on an infinite lattice are shown to qualitatively account for these effects.

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