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pith:2026:24JNQP76NNFH3DSG7II53OMC2A
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Reentrant behavior and possible $2/3$ magnetization plateau on the double-trillium langbeinite K$_2$Ni$_2$(SO$_4$)$_3$

Ivica \v{Z}ivkovi\'c, Johannes Reuther, Mat\'ias G. Gonzalez, Yurii Skourski

K2Ni2(SO4)3 shows a reentrant 2/3 magnetization plateau from a 1/3 state on the strong trillium lattice plus full polarization on the weak one.

arxiv:2605.13263 v1 · 2026-05-13 · cond-mat.str-el · cond-mat.mtrl-sci

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Claims

C1strongest claim

we reveal a signature of a 2/3 magnetization plateau consisting of a 1/3 phase on strong-TL and a fully polarized phase on weak-TL. Although in the classical limit no plateau is expected, we find a very prominent dome structure reflecting the tendency of the system to stabilize this particular spin configuration.

C2weakest assumption

The assumption that the observed magnetization feature corresponds to the proposed 1/3-plus-full polarization state and that classical Monte Carlo sufficiently captures the relevant physics for an S=1 quantum system near a spin-liquid regime.

C3one line summary

K2Ni2(SO4)3 exhibits reentrant behavior and a possible 2/3 magnetization plateau arising from a 1/3 state on the strong trillium lattice and full polarization on the weak lattice, as indicated by high-field data and classical simulations.

References

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[1] We see in Fig. 2 that the cMC calculations agree quite well with the experimental results, even though there are 4 0 50 100 150 200M (a.u.) K2Ni2(SO4)3 T = 1.50 K T = 0.80 K T = 0.57 K 0 5 10 15 20 25
[2] S. Chillal, Y. Iqbal, H. O. Jeschke, J. A. Rodriguez- Rivera, R. Bewley, P. Manuel, D. Khalyavin, P. Steffens, R. Thomale, A. T. M. N. Islam, J. Reuther, and B. Lake, Evidence for a three-dimensional 2020
[3] L. E. Chern and Y. B. Kim, Theoretical study of quan- tum spin liquids inS= 1 2 hyper-hyperkagome magnets: Classification, heat capacity, and dynamical spin struc- ture factor, Phys. Rev. B104, 094413 2021
[4] A. Fancelli, J. Reuther, and B. Lake, Classical spin models of the windmill lattice and their relevance for PbCuTe2O6, Phys. Rev. B108, 184415 (2023) 2023
[5] D. Ranaut, S. S. Shastri, S. K. Pandey, and K. Mukher- jee, Possible realization of three-dimensional quantum spin liquid behavior in HoVO4, Journal of Physics: Con- densed Matter34, 485803 (2022) 2022
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First computed 2026-05-18T02:44:49.335448Z
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d712d83ffe6b4a7d8e46fa11ddb982d03485dd604ef3fc10bdaf1ec6fc20040e

Aliases

arxiv: 2605.13263 · arxiv_version: 2605.13263v1 · doi: 10.48550/arxiv.2605.13263 · pith_short_12: 24JNQP76NNFH · pith_short_16: 24JNQP76NNFH3DSG · pith_short_8: 24JNQP76
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curl -sH 'Accept: application/ld+json' https://pith.science/pith/24JNQP76NNFH3DSG7II53OMC2A \
  | jq -c '.canonical_record' \
  | python3 -c "import sys,json,hashlib; b=json.dumps(json.loads(sys.stdin.read()), sort_keys=True, separators=(',',':'), ensure_ascii=False).encode(); print(hashlib.sha256(b).hexdigest())"
# expect: d712d83ffe6b4a7d8e46fa11ddb982d03485dd604ef3fc10bdaf1ec6fc20040e
Canonical record JSON
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