pith:6HSERTD2
Giant nonlinear optical chirality in twisted heterobilayers
Twisted MoS2/WSe2 heterobilayers produce SHG circular dichroism up to 1.96, near the theoretical maximum of 2.
arxiv:2605.17695 v1 · 2026-05-17 · physics.optics
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Claims
The magnitude of SHG circular dichroism reaches 1.96 near a 30° twist angle under 1260-nm excitation, approaching the theoretical limit of 2, with sign governed by structural handedness and reversal upon opposite incidence.
The layer-resolved model correctly isolates helicity-dependent interference between the two monolayer SHG fields without significant contributions from interface defects, strain, or higher-order effects that would alter the observed dichroism magnitude.
MoS2/WSe2 heterobilayers with controlled twist exhibit SHG circular dichroism up to 1.96, governed by structural handedness and explained by helicity-dependent interference via nonlinear Pancharatnam-Berry phase.
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Receipt and verification
| First computed | 2026-05-20T00:04:53.261710Z |
|---|---|
| Builder | pith-number-builder-2026-05-17-v1 |
| Signature | Pith Ed25519
(pith-v1-2026-05) · public key |
| Schema | pith-number/v1.0 |
Canonical hash
f1e448cc7ad5a89026ed3e91de84b5ecc463baaedf4335876665270d4ebc82a3
Aliases
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curl -sH 'Accept: application/ld+json' https://pith.science/pith/6HSERTD22WUJAJXNH2I55BFV5T \
| jq -c '.canonical_record' \
| python3 -c "import sys,json,hashlib; b=json.dumps(json.loads(sys.stdin.read()), sort_keys=True, separators=(',',':'), ensure_ascii=False).encode(); print(hashlib.sha256(b).hexdigest())"
# expect: f1e448cc7ad5a89026ed3e91de84b5ecc463baaedf4335876665270d4ebc82a3
Canonical record JSON
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