pith:RWJVYT3Z
Intertwined charge, spin, and orbital degrees of freedom under electronic correlations in the one-dimensional Fe$^{3+}$ chalcogenide chain
In the intermediate correlation regime, the Fe3+ chalcogenide chain develops an orbital-selective Mott phase where localized and itinerant electrons coexist, with no detectable pairing tendency.
arxiv:2507.09870 v3 · 2025-07-14 · cond-mat.str-el
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Claims
In the intermediate electronic correlation U/W region, an orbital-selective Mott phase with the coexistence of localized and itinerant electrons is found based on orbital-selective behavior in charge fluctuations, and no obvious pairing tendency is observed, suggesting superconductivity is unlikely to emerge in the Fe3+ systems.
The three-orbital Hubbard model derived from first-principles calculations accurately represents the low-energy physics of the real Fe3+ chain, particularly that the observed orbital-selective charge fluctuations reliably indicate a Mott phase with coexisting localized and itinerant electrons.
First-principles plus DMRG calculations on a three-orbital Hubbard model for Fe3+ chains find robust antiferromagnetic coupling, an orbital-selective Mott phase with mixed localized and itinerant electrons, and absence of pairing tendencies unlike in iron ladders.
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Receipt and verification
| First computed | 2026-06-10T01:10:56.634716Z |
|---|---|
| Builder | pith-number-builder-2026-05-17-v1 |
| Signature | Pith Ed25519
(pith-v1-2026-05) · public key |
| Schema | pith-number/v1.0 |
Canonical hash
8d935c4f799b226cef46fbc7061e60dee17ae1971ff3ebbfb87424302868c253
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Verify this Pith Number yourself
curl -sH 'Accept: application/ld+json' https://pith.science/pith/RWJVYT3ZTMRGZ32G7PDQMHTA33 \
| jq -c '.canonical_record' \
| python3 -c "import sys,json,hashlib; b=json.dumps(json.loads(sys.stdin.read()), sort_keys=True, separators=(',',':'), ensure_ascii=False).encode(); print(hashlib.sha256(b).hexdigest())"
# expect: 8d935c4f799b226cef46fbc7061e60dee17ae1971ff3ebbfb87424302868c253
Canonical record JSON
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"primary_cat": "cond-mat.str-el",
"submitted_at": "2025-07-14T02:50:40Z",
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