A fluctuation-dissipation framework derives the planar-limit Tolman length from bulk isothermal compressibility and its pressure derivative, equivalently from second and third moments of NPT volume fluctuations, yielding approximately -0.7 Å for water at 300 K.
(E12) into the leading density cou- pling (E9) gives ∆ρv = βT,vρv0 ρl0 ∆Pl + 1 2 Al βT,vβT,l ρv0 ρl0 ∆P2 l +O(∆P 3 l )
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Fluctuation-Dissipation Framework for Size-Dependent Surface Tension
A fluctuation-dissipation framework derives the planar-limit Tolman length from bulk isothermal compressibility and its pressure derivative, equivalently from second and third moments of NPT volume fluctuations, yielding approximately -0.7 Å for water at 300 K.