Arctangent-shaped ultrafast pulses enhance resonant four-wave mixing in gold nanobars through two mechanisms, phase compensation and antisymmetric polarization response, with predicted exponential gains at high harmonic orders.
S.; Rabitz, H.; Dahleh, M
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Shaping Ultrafast Pulses for Enhanced Resonant Nonlinear Interactions
Arctangent-shaped ultrafast pulses enhance resonant four-wave mixing in gold nanobars through two mechanisms, phase compensation and antisymmetric polarization response, with predicted exponential gains at high harmonic orders.