For a model H2+ molecule, short few-cycle pulses dissociate via vertical electronic excitation (VED) below about 1 fs, and via bond softening (BSD) above about 4 fs, with a smooth transition in between.
Giusti-Suzor, X
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Molecular dissociation in few-cycle laser pulses: From attosecond to femtosecond pulse duration
For a model H2+ molecule, short few-cycle pulses dissociate via vertical electronic excitation (VED) below about 1 fs, and via bond softening (BSD) above about 4 fs, with a smooth transition in between.