Electrically driven CrSBr devices emit near-infrared electroluminescence with ~94% linear polarization, and an applied magnetic field continuously shifts the emission energy by 8 meV via spin canting.
All-electrical near-field injection of excitons in a van der Waals antiferromagnet
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abstract
Van der Waals materials have become a promising building block for future electronics and photonics. The two-dimensional magnet CrSBr came into the spotlight of solid state research due to its intriguing combination of antiferromagnetic order, strong light-matter coupling and unusual quasi-1D electronic bandstructure. This study reports the electrical excitation of excitons in CrSBr layers from cryogenic temperatures up to room temperature. By exploiting the energy transfer via tunneling electrons in a graphene tunnel junction strongly bound excitons are excited in proximate CrSBr layers. This facilitates electrically-excited emission from CrSBr crystals ranging in thickness from a bilayer up to 250 nm, in which the strong linear polarization of the electroluminescence confirms the excitonic origin. For thicker layers, clear evidence for the electrically excited emission from self-hybridized exciton polaritons is observed, highlighting the strong coupling between optical excitations and confined photon modes in CrSBr. These results pave the way for future applications in spintronic and optical readout of magnetic properties.
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cond-mat.mtrl-sci 1years
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Polarized electroluminescence with magnetic spectral tuning in van der Waals magnet CrSBr
Electrically driven CrSBr devices emit near-infrared electroluminescence with ~94% linear polarization, and an applied magnetic field continuously shifts the emission energy by 8 meV via spin canting.