New criteria reveal VQE needs fault-tolerant quantum computers due to decoherence and QPE has exponentially suppressed success probability from orthogonality catastrophe in classical input states.
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Brillouin-Wigner perturbation theory plus Hartree-Fock mean-field approximation upgrades quasiparticle nuclear Hamiltonians, yielding <0.2% and ~2% ground-state energy errors versus exact shell-model results in the sd shell while preserving qubit efficiency.
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Feasibility of performing quantum chemistry calculations on quantum computers
New criteria reveal VQE needs fault-tolerant quantum computers due to decoherence and QPE has exponentially suppressed success probability from orthogonality catastrophe in classical input states.
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Improved quasiparticle nuclear Hamiltonians for quantum computing
Brillouin-Wigner perturbation theory plus Hartree-Fock mean-field approximation upgrades quasiparticle nuclear Hamiltonians, yielding <0.2% and ~2% ground-state energy errors versus exact shell-model results in the sd shell while preserving qubit efficiency.