Full quantum benchmarks show MASH agrees best with dynamics and populations in CdSe NCs, with ultrafast decay from diabatic state mixing by low-frequency phonons rather than energy relaxation.
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Full Quantum and Mixed Quantum--Classical Dynamics of Hot Exciton Cooling in Semiconductor Nanocrystals
Full quantum benchmarks show MASH agrees best with dynamics and populations in CdSe NCs, with ultrafast decay from diabatic state mixing by low-frequency phonons rather than energy relaxation.