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On-the-Fly Cavity-Molecular Dynamics of Vibrational Polaritons

physics.chem-ph · 2025-12-02 · unverdicted · novelty 7.0

An efficient parallelized on-the-fly cavity MD scheme using DFTB and beyond-long-wavelength light-matter coupling shows Mulliken charges can approximate Born charges for linear polariton spectra but cause spurious heating in energy transport studies.

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  • On-the-Fly Cavity-Molecular Dynamics of Vibrational Polaritons physics.chem-ph · 2025-12-02 · unverdicted · none · ref 5

    An efficient parallelized on-the-fly cavity MD scheme using DFTB and beyond-long-wavelength light-matter coupling shows Mulliken charges can approximate Born charges for linear polariton spectra but cause spurious heating in energy transport studies.