In Fe1/3TaS2, intercalated Fe hybridizes with Ta d-states to form a spin-polarized band that disperses along the out-of-plane direction and crosses the Fermi level, providing the interlayer magnetic-exchange channel.
Probing the anomalous Hall transport and magnetic reversal of quasi-two-dimensional antiferromagnet Co 1/3NbS2,
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Emergent 3D Fermiology and Magnetism in an Intercalated Van der Waals System
In Fe1/3TaS2, intercalated Fe hybridizes with Ta d-states to form a spin-polarized band that disperses along the out-of-plane direction and crosses the Fermi level, providing the interlayer magnetic-exchange channel.