A modified SCRAP technique using the decelerator's time-varying dc electric field as the chirp can achieve >99.5% population inversion between weak-field- and strong-field-seeking states of ammonia, improving Stark deceleration efficiency.
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Controlling rovibrational state populations of polar molecules in inhomogeneous electric fields of the Stark deceleration: molecular dynamics and quantum chemistry simulations
A modified SCRAP technique using the decelerator's time-varying dc electric field as the chirp can achieve >99.5% population inversion between weak-field- and strong-field-seeking states of ammonia, improving Stark deceleration efficiency.