A decomposition framework for dimer absorption spectra separates excitonic and charge-transfer contributions, revealing CT-induced broadening via energetic splitting rather than individual band widening, applied to a BPEA dimer.
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physics.chem-ph 2years
2026 2verdicts
UNVERDICTED 2representative citing papers
Polarization-controlled spectroscopy on conformationally flexible pentacene dimers shows persistent singlet-triplet mixing in the bound (TT1)1 state across bridging motifs, with decorrelation outcompeted by decay.
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Excitonic and Charge-Transfer Contributions to Molecular Dimer Absorption: A Decomposition Approach Applied to a BPEA Dimer
A decomposition framework for dimer absorption spectra separates excitonic and charge-transfer contributions, revealing CT-induced broadening via energetic splitting rather than individual band widening, applied to a BPEA dimer.
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Persistent singlet electronic character in the multiexcitonic triplet-pair state of strongly coupled pentacene singlet fission dimers
Polarization-controlled spectroscopy on conformationally flexible pentacene dimers shows persistent singlet-triplet mixing in the bound (TT1)1 state across bridging motifs, with decorrelation outcompeted by decay.