A pulse-shaping technique in deep UV performs coherent spectroscopy of entangled electronic-nuclear wave packets in neutral benzene, resolving 856 as electronic and 36 fs nuclear periods with coherence persisting hundreds of optical cycles.
S.et al.Molecular modes of attosecond charge migration.Phys
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Attosecond electron dynamics in molecular ions can be enhanced or suppressed by an initial charge, with the effect tied to the strength of electron correlation.
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Molecular Attoscope: Pulse Shape Spectroscopy of Electronic Coherence
A pulse-shaping technique in deep UV performs coherent spectroscopy of entangled electronic-nuclear wave packets in neutral benzene, resolving 856 as electronic and 36 fs nuclear periods with coherence persisting hundreds of optical cycles.
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Tailoring Attosecond Charge Migration in Native Molecular Ions
Attosecond electron dynamics in molecular ions can be enhanced or suppressed by an initial charge, with the effect tied to the strength of electron correlation.