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arxiv: 0802.0352 · v1 · submitted 2008-02-04 · ❄️ cond-mat.str-el · cond-mat.mtrl-sci

Spin Dynamics of Ni Cl₂-4SC(NH₂)₂ in the Field-Induced Ordered Phase

classification ❄️ cond-mat.str-el cond-mat.mtrl-sci
keywords field-inducedspinorderedphaseanisotropyantiferromagnetargueaxial
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$Ni Cl_2$-$4SC(NH_2)_2$ (known as DTN) is a spin-1 material with a strong single-ion anisotropy that is regarded as a new candidate for Bose-Einstein condensation (BEC) of spin degrees of freedom. We present a systematic study of the low-energy excitation spectrum of DTN in the field-induced magnetically ordered phase by means of high-field electron spin resonance measurements at temperatures down to 0.45 K. We argue that two gapped modes observed in the experiment can be consistently interpreted within a four-sublattice antiferromagnet model with a finite interaction between two tetragonal subsystems and unbroken axial symmetry. The latter is crucial for the interpretation of the field-induced ordering in DTN in terms of BEC.

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