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arxiv: 0806.1732 · v3 · submitted 2008-06-10 · ❄️ cond-mat.supr-con · cond-mat.str-el

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Signatures of Electronic Correlations in Optical Properties of LaFeAsO_{1-x}F_x

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classification ❄️ cond-mat.supr-con cond-mat.str-el
keywords lafeasocarrierelectronicopticalsamplesspectralsuperconductingtransfer
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Spectroscopic ellipsometry is used to determine the dielectric function of the superconducting LaFeAsO$_{0.9}$F$_{0.1}$ ($T_c$ = 27 K) and undoped LaFeAsO polycrystalline samples in the wide range 0.01-6.5 eV at temperatures 10 $\leq T \leq$ 350 K. The free charge carrier response in both samples is heavily damped with the effective carrier density as low as 0.040$\pm$0.005 electrons per unit cell. The spectral weight transfer in the undoped LaFeAsO associated with opening of the pseudogap at about 0.65 eV is restricted at energies below 2 eV. The spectra of superconducting LaFeAsO$_{0.9}$F$_{0.1}$ reveal a significant transfer of the spectral weight to a broad optical band above 4 eV with increasing temperature. Our data may imply that the electronic states near the Fermi surface are strongly renormalized due to electron-phonon and/or electron-electron interactions.

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