Doping dependence of the lattice dynamics in Ba(Fe_(1-x)Co_x)₂As₂ studied by Raman spectroscopy
classification
❄️ cond-mat.str-el
cond-mat.supr-con
keywords
splittingdopingin-planeiron-pnictidemagneticramantransitionupon
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We report Raman scattering spectra of iron-pnictide superconductor Ba(Fe$_{1-x}$Co$_x$)$_2$As$_2$ single crystals with varying cobalt $x$ content. Upon cooling through the tetragonal-to-orthorhombic transition, we observe a large splitting of the E$_g$ in-plane phonon modes involving Fe and As displacements. The splitting of the in-plane phonons at the transition is strongly reduced upon doping and disappears for $x=0.06$ qualitatively following the trend displayed by the Fe magnetic moment. The origin of the splitting is discussed in terms of magnetic frustration inherent to iron-pnictide systems and we argue that such enhanced splitting may be linked to strong spin-phonon coupling.
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