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arxiv: 1110.2936 · v2 · pith:RF2TYOC6new · submitted 2011-10-13 · ❄️ cond-mat.stat-mech

Dipolar-controlled spin tunneling and relaxation in molecular magnets

classification ❄️ cond-mat.stat-mech
keywords relaxationspinmagnetsmodelmoleculartunnelingactualapproximation
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Spin tunneling in molecular magnets controlled by dipole-dipole interactions (DDI) in the disordered state has been considered numerically on the basis of the microscopic model using the quantum mean-field approximation. In the actual case of a strong DDI spin coherence is completely lost and there is a slow relaxation of magnetization, described by t^{3/4} at short times. Fast precessing nuclear spins, included in the model microscopically, only moderately speed up the relaxation.

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