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arxiv: 1309.2916 · v1 · submitted 2013-09-10 · ❄️ cond-mat.mtrl-sci · cond-mat.str-el

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Role of doped Ru in coercivity-enhanced La_{0.6}Sr_{0.4}MnO₃ thin film studied by x-ray magnetic circular dichroism

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classification ❄️ cond-mat.mtrl-sci cond-mat.str-el
keywords magneticmomentcirculardichroismfiniteorbitalspinthin
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The coercivity of La$_{1-x}$Sr$_x$MnO$_3$ thin films can be enhanced by Ru substitution for Mn. In order to elucidate its mechanism, we performed soft x-ray absorption and magnetic circular dichroism measurements at the Ru M$_{2,3}$ and Mn L$_{2,3}$ edges. We found that the spin direction of Ru and Mn are opposite and that Ru has a finite orbital magnetic moment. Cluster-model analysis indicated that the finite orbital magnetic moment as well as the reduced spin moment of Ru result from local lattice distortion caused by epitaxial strain from the SrTiO$_3$ substrate in the presence of spin-orbit interaction.

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