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arxiv: 1601.06012 · v1 · submitted 2016-01-22 · ⚛️ physics.atom-ph · physics.atm-clus

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Electron localization in dissociating H₂^+ by retroaction of a photoelectron onto its source

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classification ⚛️ physics.atom-ph physics.atm-clus
keywords dissociatingphotoelectronbreakingelectronontoretroactionsymmetryalong
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We investigate the dissociation of $H_2^+$ into a proton and a $H^0$ after single ionization with photons of an energy close to the threshold. We find that the $p^+$ and the $H^0$ do not emerge symmetrically in case of the $H_2^+$ dissociating along the $1s\sigma_g$ ground state. Instead, a preference for the ejection of the $p^+$ in the direction of the escaping photoelectron can be observed. This symmetry breaking is strongest for very small electron energies. Our experiment is consistent with a recent prediction by Serov and Kheifets [Phys. Rev. A 89, 031402 (2014)]. In their model, which treats the photoelectron classically, the symmetry breaking is induced by the retroaction of the long range Coulomb potential onto the dissociating $H_2^+$.

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