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arxiv: 1605.09770 · v1 · pith:FYOVU4Z2new · submitted 2016-05-31 · ❄️ cond-mat.soft

Ultra-long-range dynamic correlations in a microscopic model for aging gels

classification ❄️ cond-mat.soft
keywords dynamicsagingmodelcorrelationsgelsmicroscopicparticleaccompanied
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We use large-scale computer simulations to explore the non-equilibrium aging dynamics in a microscopic model for colloidal gels. We find that gelation resulting from a kinetically-arrested phase separation is accompanied by `anomalous' particle dynamics revealed by superdiffusive particle motion and compressed exponential relaxation of time correlation functions. Spatio-temporal analysis of the dynamics reveals intermittent heterogeneities producing spatial correlations over extremely large length scales. Our study is the first microscopically-resolved model reproducing all features of the spontaneous aging dynamics observed experimentally in soft materials.

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