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arxiv: 1608.07211 · v1 · pith:R4RU4QUKnew · submitted 2016-08-25 · ⚛️ physics.atom-ph · quant-ph

Dynamics of atomic spin-orbit-state wave packets produced by short-pulse laser photodetachment

classification ⚛️ physics.atom-ph quant-ph
keywords atomicbeatslaserphotodetachmentproducedshort-pulsealignmentanalyse
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We analyse the experiment by Hultgren et al. [Phys. Rev. A {\bf 87}, 031404 (2013)] on orbital alignment and quantum beats in coherently excited atomic fine-structure manifolds produced by short-pulse laser photodetachment of C$^-$, Si$^-$ and Ge$^-$ negative ions, and derive a formula that describes the beats. Analysis of the experimental data enables us to extract the non-coherent background contribution for each species, and indicates the need for a full density matrix treatment of the problem.

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